NOLIMITS is a specialized research group and core facility at the Department of Chemistry (Faculty of Sciences), Ghent University, Belgium, founded in 2019 by Prof. Pieter Geiregat.
Our research investigates and controls ultrafast electronic and vibrational processes in materials structured on the nanometer scale. We explore how electrons, spins, phonons, and excitons evolve far from equilibrium on femtosecond time scales in novel optical materials like colloidal quantum dots, metal halide perovskites, and two-dimensional (2D) layered materials.
By pushing the frontiers of ultrafast pump-probe spectroscopy and non-linear imaging into exotic wavelength ranges—spanning the ultraviolet, visible, short-wave infrared (SWIR), mid-infrared (MIR), and terahertz (THz) domains—we uncover nonequilibrium dynamics that govern energy relaxation, charge transport, and light-matter interactions.
Colloidal Nanocrystals & Quantum Dots
Investigating ultrafast carrier dynamics, hot-carrier relaxation, and carrier trapping in direct bandgap semiconductors such as heavy-metal-free InP quantum dots, PbS nanocrystals, and colloidal quantum shells for laser gain and SWIR detection.
Metal Halide Perovskites
Revealing exciton-polaron formation, singlet-triplet annihilation, and stimulated emission thresholds in 0D, 2D, and bulk lead halide perovskite crystals and mixed-phase thin films.
2D Inorganic & Organic Materials
Studying excitonic molecules, optical Stark effects, and non-linear light-matter coupling in atomically thin 2D transition metal dichalcogenides (TMDs), CdSe nanoplatelets, and covalent organic frameworks (COFs).